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Cesium salts of manganese based lacunary phosphotungstate supported mesoporous silica: An efficient catalyst for solvent free oxidation reaction

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dc.contributor.author Rana, S.
dc.contributor.author Maddila, S.
dc.contributor.author Pagadala, R.
dc.contributor.author Parida, K.M.
dc.contributor.author Jonnalagadda, S.B.
dc.date.accessioned 2018-10-01T12:25:58Z
dc.date.available 2018-10-01T12:25:58Z
dc.date.issued 2015
dc.identifier.citation Catalysis Communications, 59, 2015: 73-77
dc.identifier.issn 1566-7367
dc.identifier.uri http://ore.immt.res.in/handle/2018/2134
dc.description School of Chemistry & Physics and the College of Agriculture, Engineering and Science, University of KwaZuluNatal, Westville campus, Durban, South Africa
dc.description.abstract Keggin-type Cs salt of Mn (II)-substituted mono-lacunary phosphotungstate supported on mesoporous silica, a novel catalyst exhibited excellent activity towards solvent free oxidation reactions. The catalyst materials were fully characterized by different techniques including XRD, BET analysis, TG-DTA, Raman spectra, FF-IR and XPS. While XPS study shown the presence of Mn (II) on the material, the existence of Keggin structure even after modification was confirmed by XRD and FT-IR data. Excellent conversion and selectivity were achieved in selective oxidation of benzyl alcohol to benzaldehyde. Optimum reaction conditions were established with respect to various parameters that influence the selective oxidation. (C) 2014 Elsevier B.V. All rights reserved.
dc.language en
dc.publisher Elsevier
dc.relation.isreferencedby SCI
dc.rights Copyright [2015]. All efforts have been made to respect the copyright to the best of our knowledge. Inadvertent omissions, if brought to our notice, stand for correction and withdrawal of document from this repository.
dc.subject Chemical Sciences
dc.title Cesium salts of manganese based lacunary phosphotungstate supported mesoporous silica: An efficient catalyst for solvent free oxidation reaction
dc.type Journal Article
dc.affiliation.author Univ KwaZulu Natal, Sch Chem & Phys, ZA-4000 Durban, South Africa


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